I mean, I'm currenty playing through Vice City stories using PPSSPP. I always loved Vice City, but never played this one since it was PSP exclusive.
The controls are utterly terrible and the 3D sometime turns borderline unwatchable, but overall I'm having a blast.
That said, I generally prefer a proper VR port rather than the same game from a VR perspective. You can probably already play GTA:SA as a floating head using VorpX or something.